Abstract: In this study, 21 small beam specimens with a pre-set through-crack were tested with FRP strips bonded to the sides to study the bond behavior between shear-strengthening FRP and concrete (referred to as “the interface” for simplicity hereafter). The test parameters included the bond length, width, thickness of FRP strip and the angle between fiber orientation and crack opening direction (referred to as “fiber tensile angle” θ hereafter) on the bond behavior of the interface. Test results showed that: 1) the small beam test setup with a pre-set crack is suitable for studying the bond behavior between FRP and concrete; 2) the bond length, width, and thickness of the FRP as well as the fiber angle have significant effects on the bond strength; 3) the distribution of FRP strains along the direction perpendicular to the fiber orientation (FRP width direction) is non-uniform; this is mainly attributed to the progressive debonding of the FRP strips in the width direction, with the FRP at the location of larger crack width debonding earlier.